Immobilization of Zinc Porphyrin Complexes on Pyridine-Functionalized Glass Surfaces

Author(s)
Agnieszka Dreas-Wlodarczak, Michael Müllneritsch, Thomas Juffmann, Carla Cioffi, Markus Arndt, Marcel Mayor
Abstract

In order to immobilize sublimable and fluorescent dye molecules on transparent surfaces for the detection of far field molecular interference experiments, we investigate the potential of pyridine-functionalized glass substrates as coordination sites for the zinc complex of tetraphenylporphyrin (ZnTPP)). Borosilicate glass is functionalized with 4-(6-(ethoxydimethylsilyl)hexyloxy)pyridine in order to cover the glass surface with pyridine subunits. ZnTPP molecules are deposited by sublimation through mechanical masks of various sizes in a high-vacuum chamber. The resulting micropatterns are analyzed using epifluorescence microscopy which also allows us to define a measure for the quality of molecular immobilization. We observe a reduced mobility and an increased efficiency for the trapping of ZnTPP on pyridine-functionalized surfaces.

Organisation(s)
Quantum Optics, Quantum Nanophysics and Quantum Information
External organisation(s)
Karlsruher Institut für Technologie, Universität Basel
Journal
Langmuir: the A C S journal of surfaces and colloids
Volume
26
Pages
10822-10826
No. of pages
5
ISSN
0743-7463
DOI
https://doi.org/10.1021/la100638u
Publication date
2010
Peer reviewed
Yes
Austrian Fields of Science 2012
103026 Quantum optics
Portal url
https://ucrisportal.univie.ac.at/en/publications/16001874-8692-4c70-b568-95715c090152