UV and VUV Ionization of Organic Molecules, Clusters, and Complexes

Author(s)
Markus Marksteiner, Philipp Haslinger, Michele Sclafani, Hendrik Ulbricht, Markus Arndt
Abstract

The generation of organic particle beams is studied in combination with

photoionization using uv radiation at 266 nm and vuv light at 157 nm.

Single-photon ionization with pulsed vuv light turns out to be sensitive enough

to detect various large neutral biomolecular complexes ranging from metal-amino

acid complexes to nucleotide clusters and aggregates of polypeptides. Different

biomolecular clusters are shown to exhibit rather specific binding

characteristics with regard to the various metals that are co-desorbed in the

source. We also find that the ion signal of gramicidin can be increased by a

factor of fifteen when the photon energy is increased from 4.66 eV to 7.9 eV.

 

Organisation(s)
Quantum Optics, Quantum Nanophysics and Quantum Information
External organisation(s)
University of Southampton
Journal
The Journal of Physical Chemistry Part A: Molecules, Spectroscopy, Kinetics, Environment and General Theory
Volume
113
Pages
9952-9957
No. of pages
6
ISSN
1089-5639
DOI
https://doi.org/10.1021/jp905039f
Publication date
2009
Peer reviewed
Yes
Austrian Fields of Science 2012
103026 Quantum optics
Portal url
https://ucrisportal.univie.ac.at/en/publications/276426da-8396-4324-86fd-9b3a0b821c81